Dynamical behavior of Borospherene: A Nanobubble

نویسندگان

  • Gerardo Martínez-Guajardo
  • José Luis Cabellos
  • Andres Díaz-Celaya
  • Sudip Pan
  • Rafael Islas
  • Pratim K. Chattaraj
  • Thomas Heine
  • Gabriel Merino
چکیده

The global minimum structure of borospherene (B40) is a cage, comprising two hexagonal and four heptagonal rings. Born-Oppenheimer Molecular Dynamics simulations show that continuous conversions in between six and seven membered rings take place. The activation energy barrier for such a transformation is found to be 14.3 kcal · mol(-1). The completely delocalized σ- and π-frameworks, as well as the conservation of the bonding pattern during rearrangement, facilitate the dynamical behavior of B40. B40 is predicted to act as a support-free spherical two-dimensional liquid at moderate temperature. In other words, B40 could be called as a nanobubble.

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عنوان ژورنال:

دوره 5  شماره 

صفحات  -

تاریخ انتشار 2015